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15. Laser-Triggered Bottom-Up Transcription of Chemical Information: Toward Patterned Graphene/MoS2 Heterostructures

Xin Chen, Mhamed Assebban, Malte Kohring, Lipiao Bao, Heiko B Weber, Kathrin C Knirsch, Andreas Hirsch – 2022

Efficiently assembling heterostructures with desired interface properties, stability, and facile patternability is challenging yet crucial to modern device fabrication. Here, we demonstrate an interface coupling concept to bottom-up construct covalently linked graphene/MoS2 heterostructures in a spatially defined manner. The covalent heterostructure domains are selectively created in analogy to the traditional printmaking technique, enabling graphic patterns at the bottom MoS2 layer to be precisely transferred to the top graphene layer. This bottom-up connection and transcription of chemical information is achieved simply via laser beam irradiation. Our approach opens up a new paradigm for heterostructure construction and integration. It enables the efficient generation and real-time visualization of spatially well-resolved covalent graphene/MoS2 heterostructures, facilitating further design and integration of patterned heterostructures into new generations of high-performance devices.

Title
15. Laser-Triggered Bottom-Up Transcription of Chemical Information: Toward Patterned Graphene/MoS2 Heterostructures
Author
Xin Chen, Mhamed Assebban, Malte Kohring, Lipiao Bao, Heiko B Weber, Kathrin C Knirsch, Andreas Hirsch
Date
2022
Identifier
doi.org/10.1021/jacs.2c00642
Citation
Journal of the American Chemical Society 2022 144 (22), 9645-9650.
Type
Text